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3 results for “Microporous Materials”
A Review on Emerging Organic-containing Microporous Material Membranes for Carbon Capture and Separation
<p><strong>Published article:</strong> Prasetya, N., Himma, N. F., Doddy Sutrisna, P., Wenten, I. G. & Ladewig, B. P. <em>Chem. Eng. J.</em> 123575 (2019). <a href="https://doi.org/10.1016/j.cej.2019.123575">https://doi.org/10.1016/j.cej.2019.123575</a></p> <p><strong>Abstract</strong></p> <p>Membrane technology has gained great attention as one of the promising strategies for carbon capture and separation. Intended for such application, membrane fabrication from various materials has been attempted. While gas separation membranes based on dense polymeric materials have been long developed, there is a growing interest to use porous materials as the membrane material. This review then focuses on emerging porous materials to be used for the fabrication of membranes that are designed for CO<sub>2</sub>separation. Criteria for selecting microporous material are first discussed, including physical and chemical properties, and parameters in membrane fabrication. Membranes based on emerging porous materials,such as metal-organic frameworks, porous organic frameworks, and microporous polymers,are then reviewed. Finally, special attention is given to recent advances, challenges, and perspectives in the development of such membranes for carbon capture and separation. </p>
Data from: Temperature-regulated guest admission and release in microporous materials
While it has long been known that some highly adsorbing microporous materials suddenly become inaccessible to guest molecules below certain temperatures, previous attempts to explain this phenomenon have failed. Here we show that this anomalous sorption behaviour is a temperature-regulated guest admission process, where the pore-keeping group's thermal fluctuations are influenced by interactions with guest molecules. A physical model is presented to explain the atomic-level chemistry and structure of these thermally regulated micropores, which is crucial to systematic engineering of new functional materials such as tunable molecular sieves, gated membranes and controlled-release nanocontainers. The model was validated experimentally with H2, N2, Ar and CH4 on three classes of microporous materials: trapdoor zeolites, supramolecular host calixarenes and metal-organic frameworks. We demonstrate how temperature can be exploited to achieve appreciable hydrogen and methane storage in such materials without sustained pressure. These findings also open new avenues for gas sensing and isotope separation.
Data from: Temperature-regulated guest admission and release in microporous materials
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