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12 results for “photolysis frequency”
Modeling actinic flux and photolysis frequencies in dense biomass burning plumes - Data asset
<p>Dataset is related to the paper by Tirpitz et al.: Modeling actinic flux and photolysis frequencies in dense biomass burning plumes</p> <p>Contains the preprocessed model input data and the modeling results (actinic fluxes and photolysis frequencies) for the Shady wildfire on July 25, 2019. The VPC model is on a private Github-Repository. Access is provided by the authors on request. See paper and INFO.txt in Data.zip for more information.</p> <p>Correspondence:<br> Jan-Lukas Tirpitz: jltirpitz@atmos.ucla.edu<br> Jochen Stutz: jochen@atmos.ucla.edu</p> <p>Other contributors:<br> Santo Fedele Colosimo<br> Nathaniel Brockway<br> Robert Spurr<br> Matthew Christi<br> Samuel Hall<br> Kirk Ullmann <br> Johnathan Hair<br> Taylor Shingler<br> Rodney Weber<br> Jack Dibb<br> Richard Moore<br> Elizabeth Wiggins<br> Vijay Natraj<br> Nicolas Theys</p>
DC3 In-Situ DC-8 Photolysis Frequency Data
DC3_jValue_AircraftInSitu_DC8_Data are photolysis rate (j value) data collected onboard the DC-8 aircraft during the Deep Convective Clouds and Chemistry (DC3) field campaign. Data collection for this product is complete.The Deep Convective Clouds and Chemistry (DC3) field campaign sought to understand the dynamical, physical, and lightning processes of deep, mid-latitude continental convective clouds and to define the impact of these clouds on upper tropospheric composition and chemistry. DC3 was conducted from May to June 2012 with a base location of Salina, Kansas. Observations were conducted in northeastern Colorado, west Texas to central Oklahoma, and northern Alabama in order to provide a wide geographic sample of storm types and boundary layer compositions, as well as to sample convection.DC3 had two primary science objectives. The first was to investigate storm dynamics and physics, lightning and its production of nitrogen oxides, cloud hydrometeor effects on wet deposition of species, surface emission variability, and chemistry in anvil clouds. Observations related to this objective focused on the early stages of active convection. The second objective was to investigate changes in upper tropospheric chemistry and composition after active convection. Observations related to this objective focused on the 12-48 hours following convection. This objective also served to explore seasonal change of upper tropospheric chemistry.In addition to using the NSF/NCAR Gulfstream-V (GV) aircraft, the NASA DC-8 was used during DC3 to provide in-situ measurements of the convective storm inflow and remotely-sensed measurements used for flight planning and column characterization. DC3 utilized ground-based radar networks spread across its observation area to measure the physical and kinematic characteristics of storms. Additional sampling strategies relied on lightning mapping arrays, radiosondes, and precipitation collection. Lastly, DC3 used data collected from various satellite instruments to achieve its goals, focusing on measurements from CALIOP onboard CALIPSO and CPL onboard CloudSat. In addition to providing an extensive set of data related to deep, mid-latitude continental convective clouds and analyzing their impacts on upper tropospheric composition and chemistry, DC3 improved models used to predict convective transport. DC3 improved knowledge of convection and chemistry, and provided information necessary to understanding the processes relating to ozone in the upper troposphere.
ATom: Actinic Flux and Photolysis Frequencies from CAFS Instrument, 2016-2018, V2
This dataset contains actinic flux and photolysis frequencies for photodissociation reactions for a variety of chemical species during the four ATom campaigns. Spectrally resolved actinic flux was measured by the down- and up-welling Charged-coupled device Actinic Flux Spectroradiometers (CAFS) from approximately 280-650 nm. Photolysis frequencies were calculated from the actinic flux and published cross sections and quantum yield values for atmospherically relevant molecules. Solar radiation drives the chemistry of the atmosphere, including the evolution of ozone, greenhouse gases, biomass burning, and other anthropogenic and natural trace constituents.
PEM Tropics B P-3B Photolysis Frequencies (J-Values)
PEM-Tropics-B_jValue_AircraftInSitu_P3B_Data is the photolysis frequencies (j-values) collected onboard the P-3B aircraft during the Pacific Exploratory Mission (PEM) Tropics B suborbital campaign. Data from the Scanning Actinic Flux Spectroradiometer (SAFS) is featured in this collection. Data collection for this product is complete.From 1983-2001, NASA conducted a collection of field campaigns as part of the Global Tropospheric Experiment (GTE). Among those was PEM, which intended to improve the scientific understanding of human influence on tropospheric chemistry. Part of the PEM field campaigns were focused on the tropical Pacific region (PEM-Tropics) which was recognized as a “very large chemical vessel.” The overarching science objective was to assess the anthropogenic impact on tropospheric oxidizing power. A secondary objective was to investigate the impact of atmospheric sulfur chemistry, including oxidation of marine biogenic emission of dimethyl sulfide (DMS) on aerosol loading and radiative effect, which is of critical importance in the assessment of global climate change. The PEM-Tropics mission was conducted in two phases to contrast the influence of biomass burning in the dry season and the “relatively clean” wet season. The first, PEM-Tropics A, was carried out during the end of the dry season (August-September 1996), and the second, PEM-Topics B, was conducted during the wet season (March-April 1999). To accomplish its objectives, PEM-Tropics enlisted the NASA DC-8 and P-3B aircrafts to carry out longitudinal and latitudinal surveys at various altitudes as well as vertical profile sampling across the Pacific basin. Both aircrafts were equipped with in-situ instruments measuring hydroperoxyl radicals (HOx), ozone (O3), photochemical precursors (including, reactive nitrogen species and non-methane hydrocarbon species), and intermediate products (e.g., hydrogen peroxide (H2O2), formaldehyde (CH2O), and acetic acid (CH3OOH). The P3-B in-situ instrument payload also included a direct measurement of hydroxyl (OH) for both missions, while the OH and hydroperoxyl radical (HO2) measurements were added to DC-8 aircraft for PEM-Tropics B. Taking advantage of its excellent low altitude capability, the P-3B was instrumented with a comprehensive sulfur measurement package and conducted pseudo-Lagragian sampling for evaluating DMS oxidation chemistry, including measurements of DMS, sulfur dioxide (SO2), sulfuric acid (H2SO4), and methylsulfonic acid (MSA) as well as the first airborne measurement of dimethyl sulfoxide (DMSO) during PEM-Tropics B. More importantly, it was the first time that DMS (the source), OH and O3 (primary oxidants), and products (DMSO, MSA, H2SO4, SO2) were measured simultaneously aboard an aircraft in the tropical pacific. These observations, specifically DMSO, presented a substantial challenge to the DMS oxidation kinetics to this day. The DC-8 aircraft was equipped with the Differential Absoprtion Lidar (DIAL) during PEM-Tropics A, and the differential absorption lidars DIAL and LASE during PEM-Tropics B. These lidars provided real-time information for fine tuning the flight tracks to capture sampling opportunities. The lidar data products themselves provide valuable information of vertical profiles of ozone as well as aerosol and water vapor in tropical Pacific Furthermore, both aircrafts were fitted with instruments for aerosol composition and microphysical property measurements. Detailed description related to the motivation, implementation, and instrument payloads are available in the PEM-Tropics A overview paper and the PEM-Tropics B overview paper. Most of the publications based on PEM-Tropics A and B observations are available in the Journal of Geophysical Research special issues: Pacific Exploratory Mission-Tropics A and NASA Global Tropospheric Experiment Pacific Exploratory Mission in the Tropics Phase B: Measurement and Analyses (PEM-Tropics B), while other publications such as Nowak et al. (2001) were published prior to the special issues.
ASIA-AQ DC-8 Photolysis Frequencies (J-Values)
ASIA-AQ_jValue_AircraftInSitu_DC8_Data is the in-situ photolysis rates collected onboard the DC-8 aircraft during the Airborne and Satellite Investigation of Asian Air Quality (ASIA-AQ) campaign. Data from the CCD-based Actinic Flux Spectroradiometer (CAFS) is featured in this collection. Data collection for this product is complete.The ASIA-AQ campaign was an international cooperative field study designed to address local air quality challenges. Conducted from January-March 2024, ASIA-AQ deployed multiple aircraft to collect in situ and remote sensing measurements, along with numerous ground-based observations and modeling assessments. Data was collected over four countries including, the Philippines, Taiwan, South Korea and Thailand and flights were conducted in full partnership with local scientists and environmental agencies responsible for air quality monitoring and assessment. One of the primary goals of ASIA-AQ was to contribute improving integration of satellite observations with existing air quality ground monitoring and modeling efforts across Asia. Air quality observations from satellites are evolving with new capabilities from South Korea’s Geostationary Environment Monitoring Spectrometer (GEMS), which conducts hourly measurements to provide a new view of air quality conditions from space that complements and depends upon ground-based monitoring efforts of countries in its field of view. ASIA-AQ science goals focused on satellite validation and interpretation, emissions quantification and verification, model evaluation, aerosol chemistry, and ozone chemistry.
POLARIS Photolysis Frequencies (J-Values)
POLARIS_jValue_AircraftInSitu_ER2_Data is the photolysis frequencies (j-values) collected during the Photochemistry of Ozone Loss in the Arctic Region in Summer (POLARIS) campaign. Data from the the Composition and Photo-Dissociative Flux Measurement (CPFM) is featured in this collection. Data collection for this product is complete.The POLARIS mission was a joint effort of NASA and NOAA that occurred in 1997 and was designed to expand on the photochemical and transport processes that cause the summer polar decreases in the stratospheric ozone. The POLARIS campaign had the overarching goal of better understanding the change of stratospheric ozone levels from very high concentrations in the spring to very low concentrations in the autumn. The NASA ER-2 high-altitude aircraft was the primary platform deployed along with balloons, satellites, and ground-sites. The POLARIS campaign was based in Fairbanks, Alaska with some flights being conducted from California and Hawaii. Flights were conducted between the summer solstice and fall equinox at mid- to high latitudes. The data collected included meteorological variables; long-lived tracers in reference to summertime transport questions; select species with reactive nitrogen (NOy), halogen (Cly), and hydrogen (HOx) reservoirs; and aerosols. More specifically, the ER-2 utilized various techniques/instruments including Laser Absorption, Gas Chromatography, Non-dispersive IR, UV Photometry, Catalysis, and IR Absorption. These techniques/instruments were used to collect data including N2O, CH4, CH3CCl3, CO2, O3, H2O, and NOy. Ground stations were responsible for collecting SO2 and O3, while balloons recorded pressure, temperature, wind speed, and wind directions. Satellites partnered with these platforms collected meteorological data and Lidar imagery. The observations were used to constrain stratospheric computer models to evaluate ozone changes due to chemistry and transport.
TRACE-P DC-8 Photolysis Frequencies (J-Values)
TRACE-P_jValue_AircraftInSitu_DC8_Data is the photolysis frequencies (j-values) measured along the DC-8 flight during the Transport and Chemical Evolution over the Pacific (TRACE-P) suborbital campaign. Data collection for this product is complete.The NASA TRACE-P mission was a part of NASA’s Global Tropospheric Experiment (GTE) – an assemblage of missions conducted from 1983-2001 with various research goals and objectives. TRACE-P was a multi-organizational campaign with NASA, the National Center for Atmospheric Research (NCAR), and several US universities. TRACE-P deployed its payloads in the Pacific between the months of March and April 2001 with the goal of studying the air chemistry emerging from Asia to the western Pacific. Along with this, TRACE-P had the objective studying the chemical evolution of the air as it moved away from Asia. In order to accomplish its goals, the NASA DC-8 aircraft and NASA P-3B aircraft were deployed, each equipped with various instrumentation. TRACE-P also relied on ground sites, and satellites to collect data. The DC-8 aircraft was equipped with 19 instruments in total while the P-3B boasted 21 total instruments. Some instruments on the DC-8 include the Nephelometer, the GCMS, the Nitric Oxide Chemiluminescence, the Differential Absorption Lidar (DIAL), and the Dual Channel Collectors and Fluorometers, HPLC. The Nephelometer was utilized to gather data on various wavelengths including aerosol scattering (450, 550, 700nm), aerosol absorption (565nm), equivalent BC mass, and air density ratio. The GCMS was responsible for capturing a multitude of compounds in the atmosphere, some of which include CH4, CH3CHO, CH3Br, CH3Cl, CHBr3, and C2H6O. DIAL was used for a variety of measurements, some of which include aerosol wavelength dependence (1064/587nm), IR aerosol scattering ratio (1064nm), tropopause heights and ozone columns, visible aerosol scattering ratio, composite tropospheric ozone cross-sections, and visible aerosol depolarization. Finally, the Dual Channel Collectors and Fluorometers, HPLC collected data on H2O2, CH3OOH, and CH2O in the atmosphere. The P-3B aircraft was equipped with various instruments for TRACE-P, some of which include the MSA/CIMS, the Non-dispersive IR Spectrometer, the PILS-Ion Chromatograph, and the Condensation particle counter and Pulse Height Analysis (PHA). The MSA/CIMS measured OH, H2SO4, MSA, and HNO3. The Non-dispersive IR Spectrometer took measurements on CO2 in the atmosphere. The PILS-Ion Chromatograph recorded measurements of compounds and elements in the atmosphere, including sodium, calcium, potassium, magnesium, chloride, NH4, NO3, and SO4. Finally, the Condensation particle counter and PHA was used to gather data on total UCN, UCN 3-8nm, and UCN 3-4nm. Along with the aircrafts, ground stations measured air quality from China along with C2H2, C2H6, CO, and HCN. Finally, satellites imagery was used to collect a multitude of data, some of the uses were to observe the history of lightning flashes, SeaWiFS cloud imagery, 8-day exposure to TOMS aerosols, and SeaWiFS aerosol optical thickness. The imagery was used to best aid in planning for the aircraft deployment.
TRACE-P P-3B Photolysis Frequencies (J-Values)
TRACE-P_jValue_AircraftInSitu_P3B_Data is the photolysis frequencies (j-values) measured along the P-3B flight aircraft during the Transport and Chemical Evolution over the Pacific (TRACE-P) suborbital campaign. Data collection for this product is complete.The NASA TRACE-P mission was a part of NASA’s Global Tropospheric Experiment (GTE) – an assemblage of missions conducted from 1983-2001 with various research goals and objectives. TRACE-P was a multi-organizational campaign with NASA, the National Center for Atmospheric Research (NCAR), and several US universities. TRACE-P deployed its payloads in the Pacific between the months of March and April 2001 with the goal of studying the air chemistry emerging from Asia to the western Pacific. Along with this, TRACE-P had the objective studying the chemical evolution of the air as it moved away from Asia. In order to accomplish its goals, the NASA DC-8 aircraft and NASA P-3B aircraft were deployed, each equipped with various instrumentation. TRACE-P also relied on ground sites, and satellites to collect data. The DC-8 aircraft was equipped with 19 instruments in total while the P-3B boasted 21 total instruments. Some instruments on the DC-8 include the Nephelometer, the GCMS, the Nitric Oxide Chemiluminescence, the Differential Absorption Lidar (DIAL), and the Dual Channel Collectors and Fluorometers, HPLC. The Nephelometer was utilized to gather data on various wavelengths including aerosol scattering (450, 550, 700nm), aerosol absorption (565nm), equivalent BC mass, and air density ratio. The GCMS was responsible for capturing a multitude of compounds in the atmosphere, some of which include CH4, CH3CHO, CH3Br, CH3Cl, CHBr3, and C2H6O. DIAL was used for a variety of measurements, some of which include aerosol wavelength dependence (1064/587nm), IR aerosol scattering ratio (1064nm), tropopause heights and ozone columns, visible aerosol scattering ratio, composite tropospheric ozone cross-sections, and visible aerosol depolarization. Finally, the Dual Channel Collectors and Fluorometers, HPLC collected data on H2O2, CH3OOH, and CH2O in the atmosphere. The P-3B aircraft was equipped with various instruments for TRACE-P, some of which include the MSA/CIMS, the Non-dispersive IR Spectrometer, the PILS-Ion Chromatograph, and the Condensation particle counter and Pulse Height Analysis (PHA). The MSA/CIMS measured OH, H2SO4, MSA, and HNO3. The Non-dispersive IR Spectrometer took measurements on CO2 in the atmosphere. The PILS-Ion Chromatograph recorded measurements of compounds and elements in the atmosphere, including sodium, calcium, potassium, magnesium, chloride, NH4, NO3, and SO4. Finally, the Condensation particle counter and PHA was used to gather data on total UCN, UCN 3-8nm, and UCN 3-4nm. Along with the aircrafts, ground stations measured air quality from China along with C2H2, C2H6, CO, and HCN. Finally, satellites imagery was used to collect a multitude of data, some of the uses were to observe the history of lightning flashes, SeaWiFS cloud imagery, 8-day exposure to TOMS aerosols, and SeaWiFS aerosol optical thickness. The imagery was used to best aid in planning for the aircraft deployment.
STRAT Photolysis Frequencies (J-Values)
STRAT_jValue_AircraftInSitu_ER2_Data is the photolysis frequencies (j-values) collected during the Stratospheric Tracers of Atmospheric Transport (STRAT) campaign. Data from the Composition and Photo-Dissociative Flux Measurement (CPFM) is featured in this collection. Data collection for this product is complete.The STRAT campaign was a field campaign conducted by NASA from May 1995 to February 1996. The primary goal of STRAT was to collect measurements of the change of long-lived tracers and functions of altitude, latitude, and season. These measurements were taken to aid with determining rates for global-scale transport and future distributions of high-speed civil transport (HSCT) exhaust that was emitted into the lower atmosphere. STRAT had four main objectives: defining the rate of transport of trace gases from the stratosphere and troposphere (i.e., HSCT exhaust emissions), improving the understanding of dynamical coupling rates for transport of trace gases between tropical regions and higher latitudes and lower altitudes (between tropical regions, higher latitudes, and lower altitudes are where most ozone resides), improving understanding of chemistry in the upper troposphere and lower stratosphere, and finally, providing data sets for testing two-dimensional and three-dimensional models used in assessments of impacts from stratospheric aviation. To accomplish these objectives, the STRAT Science Team conducted various surface-based remote sensing and in-situ measurements. NASA flew the ER-2 aircraft along with balloons such as ozonesondes and radiosondes just below the tropopause in the Northern Hemisphere to collect data. Along with the ER-2 and balloons, NASA also utilized satellite imagery, theoretical models, and ground sites. The ER-2 collected data on HOx, NOy, CO2, ozone, water vapor, and temperature. The ER-2 also collected in-situ stratospheric measurements of N2O, CH4, CO, HCL, and NO using the Aircraft Laser Infrared Absorption Spectrometer (ALIAS). Ozonesondes and radiosondes were also deployed to collect data on CO2, NO/NOy, air temperature, pressure, and 3D wind. These balloons also took in-situ measurements of N2O, CFC-11, CH4, CO, HCL, and NO2 using the ALIAS. Ground stations were responsible for taking measurements of O3, ozone mixing ratio, pressure, and temperature. Satellites took infrared images of the atmosphere with the goal of aiding in completing STRAT objectives. Pressure and temperature models were created to help plan the mission.
PEM Tropics A DC-8 Photolysis Frequencies (J-Values)
PEM-Tropics-A_jValue_AircraftInSitu_DC8_Data is the photolysis frequencies (j-values) measured along the DC-8 flight during the Pacific Exploratory Mission (PEM) Tropics A suborbital campaign. Data collection for this product is complete.From 1983-2001, NASA conducted a collection of field campaigns as part of the Global Tropospheric Experiment (GTE). Among those was PEM, which intended to improve the scientific understanding of human influence on tropospheric chemistry. Part of the PEM field campaigns were focused on the tropical Pacific region (PEM-Tropics) which was recognized as a “very large chemical vessel.” The overarching science objective was to assess the anthropogenic impact on tropospheric oxidizing power. A secondary objective was to investigate the impact of atmospheric sulfur chemistry, including oxidation of marine biogenic emission of dimethyl sulfide (DMS) on aerosol loading and radiative effect, which is of critical importance in the assessment of global climate change. The PEM-Tropics mission was conducted in two phases to contrast the influence of biomass burning in the dry season and the “relatively clean” wet season. The first, PEM-Tropics A, was carried out during the end of the dry season (August-September 1996), and the second, PEM-Topics B, was conducted during the wet season (March-April 1999). To accomplish its objectives, PEM-Tropics enlisted the NASA DC-8 and P-3B aircrafts to carry out longitudinal and latitudinal surveys at various altitudes as well as vertical profile sampling across the Pacific basin. Both aircrafts were equipped with in-situ instruments measuring hydroperoxyl radicals (HOx), ozone (O3), photochemical precursors (including, reactive nitrogen species and non-methane hydrocarbon species), and intermediate products (e.g., hydrogen peroxide (H2O2), formaldehyde (CH2O), and acetic acid (CH3OOH). The P3-B in-situ instrument payload also included a direct measurement of hydroxyl (OH) for both missions, while the OH and hydroperoxyl radical (HO2) measurements were added to DC-8 aircraft for PEM-Tropics B. Taking advantage of its excellent low altitude capability, the P-3B was instrumented with a comprehensive sulfur measurement package and conducted pseudo-Lagragian sampling for evaluating DMS oxidation chemistry, including measurements of DMS, sulfur dioxide (SO2), sulfuric acid (H2SO4), and methylsulfonic acid (MSA) as well as the first airborne measurement of dimethyl sulfoxide (DMSO) during PEM-Tropics B. More importantly, it was the first time that DMS (the source), OH and O3 (primary oxidants), and products (DMSO, MSA, H2SO4, SO2) were measured simultaneously aboard an aircraft in the tropical pacific. These observations, specifically DMSO, presented a substantial challenge to the DMS oxidation kinetics to this day. The DC-8 aircraft was equipped with the Differential Absoprtion Lidar (DIAL) during PEM-Tropics A, and the differential absorption lidars DIAL and LASE during PEM-Tropics B. These lidars provided real-time information for fine tuning the flight tracks to capture sampling opportunities. The lidar data products themselves provide valuable information of vertical profiles of ozone as well as aerosol and water vapor in tropical Pacific Furthermore, both aircrafts were fitted with instruments for aerosol composition and microphysical property measurements. Detailed description related to the motivation, implementation, and instrument payloads are available in the PEM-Tropics A overview paper and the PEM-Tropics B overview paper. Most of the publications based on PEM-Tropics A and B observations are available in the Journal of Geophysical Research special issues: Pacific Exploratory Mission-Tropics A and NASA Global Tropospheric Experiment Pacific Exploratory Mission in the Tropics Phase B: Measurement and Analyses (PEM-Tropics B), while other publications such as Nowak et al. (2001) were published prior to the special issues.
PEM Tropics B DC-8 Photolysis Frequencies (J-Values)
PEM-Tropics-B_TraceGas_AircraftInSitu_DC8_Data is the photolysis frequencies (j-values) collected onboard the DC-8 aircraft during the Pacific Exploratory Mission (PEM) Tropics B suborbital campaign. Data collection for this product is complete.From 1983-2001, NASA conducted a collection of field campaigns as part of the Global Tropospheric Experiment (GTE). Among those was PEM, which intended to improve the scientific understanding of human influence on tropospheric chemistry. Part of the PEM field campaigns were focused on the tropical Pacific region (PEM-Tropics) which was recognized as a “very large chemical vessel.” The overarching science objective was to assess the anthropogenic impact on tropospheric oxidizing power. A secondary objective was to investigate the impact of atmospheric sulfur chemistry, including oxidation of marine biogenic emission of dimethyl sulfide (DMS) on aerosol loading and radiative effect, which is of critical importance in the assessment of global climate change. The PEM-Tropics mission was conducted in two phases to contrast the influence of biomass burning in the dry season and the “relatively clean” wet season. The first, PEM-Tropics A, was carried out during the end of the dry season (August-September 1996), and the second, PEM-Topics B, was conducted during the wet season (March-April 1999). To accomplish its objectives, PEM-Tropics enlisted the NASA DC-8 and P-3B aircrafts to carry out longitudinal and latitudinal surveys at various altitudes as well as vertical profile sampling across the Pacific basin. Both aircrafts were equipped with in-situ instruments measuring hydroperoxyl radicals (HOx), ozone (O3), photochemical precursors (including, reactive nitrogen species and non-methane hydrocarbon species), and intermediate products (e.g., hydrogen peroxide (H2O2), formaldehyde (CH2O), and acetic acid (CH3OOH). The P3-B in-situ instrument payload also included a direct measurement of hydroxyl (OH) for both missions, while the OH and hydroperoxyl radical (HO2) measurements were added to DC-8 aircraft for PEM-Tropics B. Taking advantage of its excellent low altitude capability, the P-3B was instrumented with a comprehensive sulfur measurement package and conducted pseudo-Lagragian sampling for evaluating DMS oxidation chemistry, including measurements of DMS, sulfur dioxide (SO2), sulfuric acid (H2SO4), and methylsulfonic acid (MSA) as well as the first airborne measurement of dimethyl sulfoxide (DMSO) during PEM-Tropics B. More importantly, it was the first time that DMS (the source), OH and O3 (primary oxidants), and products (DMSO, MSA, H2SO4, SO2) were measured simultaneously aboard an aircraft in the tropical pacific. These observations, specifically DMSO, presented a substantial challenge to the DMS oxidation kinetics to this day. The DC-8 aircraft was equipped with the Differential Absoprtion Lidar (DIAL) during PEM-Tropics A, and the differential absorption lidars DIAL and LASE during PEM-Tropics B. These lidars provided real-time information for fine tuning the flight tracks to capture sampling opportunities. The lidar data products themselves provide valuable information of vertical profiles of ozone as well as aerosol and water vapor in tropical Pacific Furthermore, both aircrafts were fitted with instruments for aerosol composition and microphysical property measurements. Detailed description related to the motivation, implementation, and instrument payloads are available in the PEM-Tropics A overview paper and the PEM-Tropics B overview paper. Most of the publications based on PEM-Tropics A and B observations are available in the Journal of Geophysical Research special issues: Pacific Exploratory Mission-Tropics A and NASA Global Tropospheric Experiment Pacific Exploratory Mission in the Tropics Phase B: Measurement and Analyses (PEM-Tropics B), while other publications such as Nowak et al. (2001) were published prior to the special issues.
SASS (Subsonics Assessment) Ozone and NOx Experiment (SONEX) Photolysis Frequencies (J-Values)
SONEX_jValue_AircraftInSitu_DC8_Data_1 is the photolysis frequencies (j-values) measured along the DC-8 flight by the Scanning Actinic Flux Spectroradiometers (SAFS). Data collection is complete.The SASS (Subsonics Assessment) Ozone and NOx Experiment (SONEX) was an international, multi-organizational mission that took place in October-November 1997. NASA was the US sponsor of SONEX that partnered with POLINAT-2 (Pollution from Aircraft Emissions in the North Atlantic Flight Corridor) funded by the German DLR (Deutsches Zentrum für Luft- und Raumfahrt) or German Aerospace Agency. NASA flew the DC-8 aircraft out of NASA/Ames Research Center. DLR operated an instrumented Falcon 20 aircraft. The staging locations for NAFC sampling were primarily Bangor, Maine (US), and Shannon, Ireland. Subsonic aircraft emissions impact several aspects of atmospheric composition: nitrogen oxides (NOx), CO, and hydrocarbons from emissions can perturb upper tropospheric/lower stratospheric (UT/LS) ozone; water vapor, soot, and sulfur oxides (SOx) emitted by aircraft may perturb clouds and aerosols, changing UT/LS radiative forcing and global temperature.In SONEX and POLINAT, flights were conducted in the vicinity of the North Atlantic Flight Coordinator (NAFC) to observe the impact of aircraft emissions on NOx and ozone (O3). The DC-8 aircraft payload (Singh et al., 1999) primarily measured in-situ CO, CO2, hydrocarbons/halocarbons, O3, aerosols (Dibb et al., 2000), OH/HO2, water vapor, nitric acid (Talbot et al., 1999), photolysis rates, temperature, pressure, winds, NOx, and NOy.Three sampling approaches were implemented during SONEX. First, special meteorological (Fuelberg et al., 2000) were developed to allow targeted sampling for air parcels affected by aircraft emissions and various meteorological events, e.g., convection, lightning (Jeker et al., 2000), stratospheric intrusions (Cho et al., 2000). Second, because the NAFC had not been extensively sampled in the past, it was important for SONEX to characterize the climatology of trace species like CN (Wang et al., 2000), NOx and NOy (Koike et al., 2000). Third, tracers (Simpson et al., 2000; Thompson et al., 1999) and model sensitivity studies (Meijer et al., 2000) were employed for Air Mass Identification. This sampling strategy answered the following questions: Where and when are air masses found with the greatest aircraft influence? When and where was stratospheric air sampled? SONEX showed a substantial impact of aircraft emissions on UT/LS NOx and CN in the vicinity of fresh aircraft emissions. However, during October-November 1997 over the NAFC, UT/LS NOx was dominated by surface emissions redistributed by convection and augmented by lightning.
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