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2 results for “iodine monoxide”
Iodine monoxide (IO) measurements made using a MAX-DOAS (Multi-AXis Differential Optical Absorption Spectroscopy) instrument in the austral summer of 2016/17 during the Antarctic Circumnavigation Expedition (ACE).
<p><strong>Dataset abstract</strong></p> <p>To achieve the objectives of the project, we installed a MAX-DOAS (Multi-AXis Differential Optical Absorption Spectroscopy) instrument on the vessel “Akademik Tryoshnikov”. This instrument is based on the DOAS technique, which is used to measure trace gas concentrations in the atmosphere. The method consists of the analysis of the spectral absorption lines that each trace gas produces in the solar spectra. The DOAS technique uses the narrowband features that every trace gas has in their spectral absorption coefficients. This differential cross section is unique and acts like a fingerprint for the trace gases, allowing to differentiate between them and to estimate their concentrations (for further details see Platt and Stutz, 2008).</p> <p>In the past decades, atmospheric chemists have come to realize that halogen species (like Cl, Br or I and their oxides ClO, BrO and IO) exert a powerful influence on the chemical composition of the troposphere and through that influence affect the evolution of pollutants, hence having a significant impact on climate. These reactive halogen species are potent oxidizers for organic and inorganic compounds throughout the troposphere. In particular, halogen cycles can act on several compounds (such as methane, ozone, particles…), all of which are climate forcing agents through direct and indirect radiative effects. Dynamic exchange of halogens between ocean, sea ice, snowpack and atmosphere is the main driver for the frequent occurrence of Ozone Depletion Events (ODEs) and Atmospheric Mercury Depletion Events (AMDEs) (Saiz-Lopez and von Glasow, 2012).</p> <p>In this dataset we present the mixing ratio and vertical column density of iodine monoxide (IO) recorded in the austral summer of 2016/2017 in the Southern Ocean and Atlantic Ocean, averaged over one-hour time periods.</p> <p><strong>Dataset contents</strong></p> <ul> <li>ace_iodine_monoxide_atmospheric_measurements.csv, data file, comma-separated values</li> <li>data_file_header.txt, metadata, text</li> <li>README.pdf, metadata, PDF/A1-a</li> <li>README.txt, metadata, text</li> </ul> <p><strong>Dataset license</strong></p> <p>This dataset of atmospheric iodine monoxide measurements from ACE is made available under the Creative Commons Attribution 4.0 International License (CC BY 4.0) whose full text can be found at https://creativecommons.org/licenses/by/4.0/</p>
Measurements and model simulations of iodine monoxide (IO) radical, water vapor (H2O), nitrogen dioxide (NO2) radical, formaldehyde (HCHO), gaseous elemental mercury (Hg0), and oxidized mercury (HgII) at Storm Peak Laboratory, Colorado, during April 2022
<p>This dataset was compiled to accompany the manuscript Lee et al., titled "Elevated Tropospheric Iodine over the Central Continental United States: Is Iodine a Major Oxidant of Atmospheric Mercury?", submitted to <em>AGU Geophysical Research Letters</em>.</p> <p> </p> <p><strong>file01</strong> contains two example spectral proofs for iodine monoxide (IO) radical measured by the University of Colorado Multi-AXis Differential Optical Absorption Spectroscopy (CU MAX-DOAS) instrument at Storm Peak Laboratory, CO (SPL; 3220 meters above sea level; 40.455 degrees North; 106.745 degrees West) during April 2022.</p> <p><strong>file02</strong> contains oxygen collision-induced absorption (O2-O2) slant column densities (SCDs) measured in a spectral fit window from 350 to 388 nm by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file03</strong> contains O2-O2 SCDs measured in a spectral fit window from 425 to 490 nm by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file04</strong> contains IO SCDs measured in a spectral fit window from 417.5 to 438 nm by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file05</strong> contains water vapor (H2O) SCDs measured in a spectral fit window from 425 to 490 nm by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file06</strong> contains nitrogen dioxide (NO2) radical SCDs measured in a spectral fit window from 425 to 490 nm by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file07</strong> contains formaldehyde (HCHO) SCDs measured in a spectral fit window from 328,5 to 359 nm by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file08</strong> contains the profiles of pressure, temperature, O2-O2, ozone (O3), NO2, and H2O derived from ECMWF CAMS reanalysis (April 2022 at SPL) and used in the radiative transfer model McArtim3 to calculate weighting functions for the trace gas profile inversions of IO, H2O, NO2, and HCHO.</p> <p><strong>file09</strong> contains the a priori profiles used for the IO profile inversions during April 2022 at SPL. One profile assumes a "flat" profile shape with a constant volume mixing ratio of 0.10 pptv throughout the atmosphere. The other profile is adapted from the GEOS-Chem April 2022 daytime (SZA < 85) average.</p> <p><strong>file10</strong> contains the a priori profile used for the H2O profile inversions during April 2022 at SPL. The profile is adapted from the GEOS-Chem April 2022 daytime (SZA < 85) average.</p> <p><strong>file11</strong> contains the a priori profile used for the NO2 profile inversions during April 2022 at SPL. The profile is adapted from the GEOS-Chem April 2022 daytime (SZA < 85) average.</p> <p><strong>file12</strong> contains the a priori profile used for the HCHO profile inversions during April 2022 at SPL. The profile is adapted from the GEOS-Chem April 2022 daytime (SZA < 85) average.</p> <p><strong>file13</strong> contains the IO tropospheric vertical column densities (VCDtrop; surface to 12 km), volume mixing ratios near instrument altitude (VMRinstr), and degrees of freedom (DoF) measured by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file14</strong> contains the H2O VCDtrop, VMRinstr, and DoF measured by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file15</strong> contains the NO2 VCDtrop, VMRinstr, and DoF measured by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file16</strong> contains the HCHO VCDtrop, VMRinstr, and DoF measured by the CU MAX-DOAS instrument at SPL from April 1 to April 30, 2022.</p> <p><strong>file17</strong> contains GEOS-Chem simulated temperature, relative humidity, IO VCDtrop & VMRinstr, H2O VCDtrop & VMRinstr, NO2 VCDtrop & VMRinstr, HCHO VCDtrop & VMRinstr, and bromine monoxide (BrO) radical VCDtrop & VMRinstr at SPL from April 1 to April 30, 2022.</p> <p><strong>file18</strong> contains the gaseous elemental mercury (Hg0) measured by the Utah State University dual-channel mercury system at SPL from April 1 to April 30, 2022.</p> <p><strong>file19</strong> contains the oxidized mercury (HgII) measured by the Utah State University dual-channel mercury system at SPL from April 1 to April 30, 2022.</p> <p><strong>file20</strong> contains the GEOS-Chem simulated Hg0 and HgII at SPL from April 1 to April 30, 2022.</p> <p><strong>file21</strong> contains the profiles of pressure, temperature, relative humidity, BrO, bromine atom (Br), methane (CH4), chlorine monoxide (ClO) radical, chlorine atom (Cl), carbon monoxide (CO), Hg0, peroxy radical (HO2), IO, iodine atom (I), NO2, hydroxyl radical (OH), and O3 used as constraints for the gas-phase mercury box model. All profiles except IO and I are adapted from the GEOS-Chem April 2022 daytime (SZA < 85) average. The IO profile was calculated by scaling the GEOS-Chem April 2022 daytime (SZA < 85) average below 12 km by the average observed IO VCDtrop during April 2022. The I atom profile was calculated by multiplying the scaled IO profile by the ratio of unscaled I / unscaled IO profiles from GEOS-Chem.</p> <p> </p> <p><strong>file22</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file23</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file24</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file25</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file26</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file27</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file28</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file29</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file30</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file31</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file32</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file33</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file34</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file35</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file36</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file37</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file38</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file39</strong> contains the time-resolved gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p> </p> <p><strong>file40</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file41</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file42</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file43</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file44</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file45</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file46</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file47</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file48</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgOH</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file49</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file50</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file51</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at half the rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file52</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file53</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file54</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at the same rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file55</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>8 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file56</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>9.5 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p> <p><strong>file57</strong> contains a profile of the gas-phase mercury box model output assuming that <strong>HgI forms at twice the rate as HgBr</strong> and that the Hg-I bond strength is <strong>11 kcal / mol</strong>, using <strong>HgBr</strong> as reference for the B-value in the HgI equilibrium coefficient.</p>
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